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Time-dependent density functional theory (TDDFT) has seen a surge ofapplications in recent years, for the calculation of optical spectra andresponse of atoms, molecules, clusters, and solids. But TDDFT notlimited to the linear response regime; its promise to describe electroncorrelation in strong-field phenomena, including high-harmonicgeneration, above-threshold ionization, and electronic quantum controltheory, is only beginning to be tapped. The non-perturbative regime iswhere TDDFT is the only feasible scheme, as wavefunction methods foreven a few electrons are prohibitively expensive.Although in principle an exact theory, the functionals of TDDFT must inpractise be approximated. I will discuss certain properties of the exactfunctional that are essential for approximations to satisfy in order tocapture the dynamics accurately in strong fields. Some of these areparticularly challenging to incorporate into functional approximations,for example history-dependence and initial-state-dependence, criticalfor attosecond quantum control phenomena. I will present a new extensionto phase-space density functionals, which may turn out to be a morenatural framework for these problems.Begin streaming QuickTime of the whole talk (high bandwidth).(Or, right-click to download the movie.)(Or, right-click to download the podcast.)Begin streaming RealMedia for the whole talk: high bandwidth or medium bandwidth.Or, stream audio only for the whole talk:high bandwidth or low bandwidth.(Or, right-click to download the whole audio file.)To begin viewing slides, click on the first slide below.(Or, view as pdf.) Author entry (protected)
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